I.
INTRODUCTION
Thermal rectification (TR) [1, 2] is an important property that has been extensively studied in a variety of
nonlinear systems [312] in recent times. A thermally
driven system can be so designed such that the thermal
current through the system has unequal values when direction of thermal bias is reversed - the heat conduction
is asymmetric. Thus the system behaves as a good heat
conductor in one direction and a good insulator in the opposite direction. Thermal rectification owes its origin to
the nonlinearity of the system and to its spatial asymmetry. Analogous to its electrical counterpart, the thermal
rectifier is considered to be a crucial building block and
therefore has an important role to play in the fabrication
of sophisticated thermal devices.
Negative differential thermal resistance (NDTR) [1, 2]
is a counter intuitive phenomenon, predicted in the heat
conduction studies, where the steady state thermal current decreases as the temperature difference across a system is increased. In the recent decades a lot of attention has been devoted to study NDTR in nonlinear lattices. However, in spite of enormous efforts the underlying physical mechanism that generates NDTR in nonlinear system is still not satisfactorily understood. A lot
of mechanisms have been proposed and many unresolved
questions regarding the emergence of NDTR, such as the
mismatch of the phonon bands [13, 14], role of interface
[15], ballistic-diffusive transport [16, 17], role of momentum conservation [18] presence of a critical system size
and a transition from the exhibition to the nonexhibition
of NDTR [19] and scaling [20] are still being explored.
NDTR is considered to be of immense technological im-
address: debarshee.bagchi@saha.ac.in
portance in the working of recently proposed thermal devices such as the thermal transistors [13], thermal logic
gates [14], thermal memory elements [21] etc. Theoretical studies using mostly numerical simulation have been
employed extensively to study both these feature in many
nonlinear lattice systems, few examples are the FrenkelKontorova model [6, 19], the 4 model [15], the FermiPasta-Ulam chain [7, 18], the Morse lattice [5].
Linear systems, such as the coupled harmonic oscillators, do not exhibit TR or NDTR. Surprisingly it has
been recently found that linear graded systems, such as a
harmonic oscillator chain with linearly increasing masses,
show both TR and NDTR [8, 9]. In fact, gradual massloaded carbon and boron nitride nanotubes have already
been used effectively to fabricate a thermal rectifier [22].
These functional graded materials have been considered
to be of huge technological relevance since these materials
can be purposely manufactured and have many intriguing optical, electrical, mechanical and thermal properties
[8].
Motivated by the concept of these functional graded
materials, in this paper, we study thermal transport in
the classical Heisenberg model [23, 24] coupled to heat
baths and in presence of a spatially varying magnetic
field, and investigate TR and NDTR. Both of these features have been shown to emerge in the Heisenberg spin
chain previously [25] but by a different approach; in this
paper we present a new route to obtain these features.
Investigation of TR and NDTR in spin systems have
been carried out only in a very few other works such
as the two dimensional classical Ising model [26] and
quantum spin systems [27] very recently. These systems
are quite simple and although they are helpful in understanding the underlying physical mechanism, nevertheless these are not very realistic; the Heisenberg model is
a comparatively more realistic spin model for a magnetic
insulator. Also, in both cases the system under consider-
2
ation consists of two dissimilar segments coupled to each
other. This scheme requires one to carefully fabricate the
junction as it has been argued that TR and NDTR are
crucially dependent on the junction properties [17, 19]
which is difficult to implement this in real systems. It
was also initially believed that NDTR can not be obtained in a symmetric system [28]. However later studies
clearly showed that NDTR can be obtained from systems
even without structural inhomogeneity [20, 29].
The advantage of our proposal is that it is much simpler to implement, easy to manipulate over a wide range,
and should also be realizable in practice. Firstly, one
does not need to specially design the system, unlike the
case of two segment nonlinear lattices (with an interface)
or graded systems mentioned above - one has to fabricate
such a system with precise specifications which might be
technologically more challenging and restrictive in applicability. Secondly, using spin systems one can control TR
and NDTR over a wide range by tuning only an external
magnetic field and so, in contrast to previous works, no
special engineering of the system is required in our case.
TR in this system also shows interesting anomalous dependences, as we shall discuss, that can be of technological relevance.
The organization of the rest of the paper is as follows.
In the next section Sec II we describe our model and the
numerical scheme employed to study the system. Thereafter we present our results in Sec. III. Finally, in Sec
IV we conclude with a brief summary of our results and
a discussion.
II.
Consider classical Heisenberg spins {S~i } (threedimensional unit vectors) on a one-dimensional lattice of
length N (1 i N ) with nearest neighbor interaction.
The Hamiltonian of the system is
H = K
N
1
X
~i S
~i+1
S
i=1
N
X
~hi S
~i
(1)
i=1
where the spin-spin interaction are taken to interact ferromagnetically K > 0 (we have set K to unity for our
results without any loss of generality). The second term
in Eq. (1) is due to a spatially varying magnetic field
~hi that acts on all the spins. The equation for the time
evolution of the spin vectors can be written as
d~
~i B
~i
Si = S
dt
(2)
~i = S
~i1 + S
~i+1 + ~hi (with K = 1) is the local
where B
molecular field experienced by i-th spin vector.
To drive the system out of equilibrium we couple the
ends of the system to two heat baths. This is implemented by introducing to additional spins at sites
~0 , S
~1 ) and
i = 0 and i = N + 1. The bonds between (S
~N , S
~N +1 ) at two extreme ends of the system behave
(S
as stochastic thermal baths. The left and right thermal baths are in equilibrium at their respective tempera~0 S
~1
tures, Tl and Tr and the bond energies El = S
~
~
and Er = SN SN +1 have Boltzmann distribution
P (E) exp(E/T ). The average energies of the two extreme bonds read hEl i = L(Tl1 ) and hEr i = L(Tr1 ),
L(x) = coth(x) 1/x being the standard Langevin function.
We investigate the steady state transport properties
of the Heisenberg model by numerically computing the
steady state thermal current using the discrete time odd
even (DTOE) dynamics [25, 30]. The DTOE dynamics
alternately updates the spins belonging to the odd and
even sites of the lattice using a spin precession dynamics
given by
h
i
~i,t+1 = S
~ cos + (S
~ B)
sin + (S
~ B)
B(1
cos )
S
i,t
(3)
i = B
~ i /|B
~ i |, i = |B
~ i |t and t is the time-step
where B
increment [30].
~0 is updated with the
Numerically, the leftmost spin S
~N +1 is updated with
even spins and the rightmost spin S
the odd (even) spins for even (odd) N . The bond energy
~0 and S
~1 is refreshed from a Boltzmann distribetween S
~0 is reconstructed using
bution and thereafter the spin S
~0 S
~1 . Note that, during this update
the relation E0 = S
~1 is not modified (as it belongs to the odd sublattice).
S
Similarly the other end is also updated. This sets the
temperatures of the two ends of the lattice to our desired
values. A thorough discussion of the DTOE scheme and
numerical implementation of the thermal baths can be
found in Ref. [30].
The computation of the steady state thermal current is
done as described in the following. The energy of the i-th
bond Eio measured after the odd spin update is not equal
to Eie measured after
the subsequent
even spin update,
i
h
~
~i S
~i+1 + hi is the energy density. This
where Ei = S
(4)
3
RESULTS
= 0.1
= 0.3
= 0.5
= 0.7
= 0.9
1.5
Thermal Rectification
30
20
10
0
-10
-20
-30
-40
-50
= 0.5
= 1.0
= 1.5
= 2.0
(a)
1.8
= 0.5
= 1.0
= 1.5
= 2.0
-1
-0.5
0.5
J , J-
1.6
1.4
(b)
1.2
1
1
0.2
0.4
0.6
0.8
An interesting feature of TR in this system is the variation of the rectification ratio R = |J /J | with the
parameter . The rectification ratio does not increase indefinitely as is increased but rather shows an intriguing
nonmonotonic dependence. For different values of the
thermal bias we compute R as a function of and
is shown in Fig. 2a. For in the range 0 < <
0 , we
find R > 1 initially whereas for >
,
R
<
0 1, where
0 lies roughly in the range 3.5 < < 4.0 (Fig. 2a).
For small , R increases roughly linearly for < 0 ,
then drops abruptly below R = 1 and then increases
1
(a)
0.5
0
1.8
1.6
1.4
1.2
1
0.8
0.6
0.4
0.2
T = 0.5
= 1.0
= 1.5
= 2.0
(b)
0
A.
III.
1.8
1.6
1.4
1.2
1
0.8
0.6
0.4
0.2
N = 100
= 200
= 500
= 1000
(c)
0
5
12345367895
8
5 45367895
102
= 0.9
10
100
= 0.1
10-1
10
10-3
= 1.0
= 2.0
100
10-1
(a)
-2
T = 0.5
101
J
J , |J-|
10-2
(b)
0
10-1
N = 200
10-2
J / N
= 500
= 1000
10-3
10-4
(c)
-5
10
FIG. 4. (Color online) (a) Variation of the individual currents J and |J | with for two values of the thermal
gradient = 0.1 and 0.9. Average temperatures T = 1.0.
(b) Variation of J with for different average temperatures
T = 0.5, 1.0 and 2.0. Here = 0.5 and N = 500 in both
the cases. (c) Variation of J (scaled by N ) with for different system size N = 200, 500 and 1000. Here T = 1.0 and
= 0.5. For (b) and (c) |J | has similar variation as in (a).
5
1
<Sz>, <Sz>-
(a)
0.8
0.6
(b)
0.4
-1
0
Sz
0.5
2.4
<Sz>
<Sz>-
1.6
T = 1.0
= 2.0
1.2
N = 500
= 100
1.6
6
3
2.8
2.6
2.4
2.2
2
1.8
-1
15
-1
5
(c)
0
0
(c)
20
2.8
15
10
3.2
20
-1, --1
-0.5
(b)
2.8
2.4
-6
10
3.2
(a)
2.8
PN(Sz)
-5
10
3.2
= 1.0
= 3.0
= 5.0
-3
10
= 7.0
-4
10
-2
10
-1
10
2.4
10
(d)
= 0.5
= 0.9
1.6
5
0
6 0
6
the passage of energy in the bulk of the system which is
required in order to observe NDTR [25].
0.4
= 1.7
= 1.8
= 1.9
= 2.0
= 2.2
h0 = 1.6
= 1.7
= 1.8
0.8
= 2.0
0.6
= 2.2
1
0.4
0.2
0.2
(a)
0
0
0.1
0.2
0.3
0.4
(b)
0.5
0.1
0.2
0.3
0.4
0.5
(a)
1.2
1
(b)
0.8
J/Jm
0.6
0.4
0.6
J / T2
0.6
0.8
0.2
0.4
0.6
N = 100
= 500
= 1000
0.4
0.2
0
-0.6
-0.4
-0.2
( - m) / T
0.2
0.2
0
0.1
0.2
0.3
0.4
DISCUSSION
To summarise our main results, we have studied thermal rectification (TR) and negative differential thermal resistance (NDTR) in the one dimensional classical Heisenberg model under thermal bias with a spatially varying magnetic field. Systematic analysis of TR
with respect to system parameters reveal intriguing dependences with respect to temperature and system size.
For certain range of system parameters NDTR can be
observed. Both the features emerge and can be controlled by the external magnetic field unlike the previous works where one had to prepare the system with
specific parameter values. Heat transport in magnetic
system assisted by classical spin waves have been predicted several years back [31] and has also been experimentally observed recently in yttrium iron garnet
[32, 33]. Transport studies in spin systems are also of
active experimental interest in recent times [34, 35]. Actual chemical compounds [3638] that mimic classical
spin interactions, such as TMMC((CH3 )4 NMnCl3 ) and
DMMC((CH3 )2 NH2 MnCl3 ), are already known for quite
some time now. Apart from carbon nanotubes which are
considered suitable for fabricating thermal devices, this
present work (and also [25]) suggests these spin materials to be another promising candidate. Hopefully, with
the recent advancement in low dimensional experimental
techniques, these theoretical predictions would be verified experimentally and lead to the efficient thermal management in future.
0.5
7
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