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Construction and Building Materials 163 (2018) 122–138

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Construction and Building Materials


journal homepage: www.elsevier.com/locate/conbuildmat

Assessment of gamma radiation shielding properties of concrete


containers containing recycled coarse aggregates
Dahee Han a,⇑, Woojae Kim b, Sangkyu Lee c, Hakyoung Kim d, Pedro Romero a
a
Department of Civil and Environmental Engineering, University of Utah, Salt Lake City, USA
b
POSCO E&C, 6F, OIC Building, POSCO Global R&D Center, 100, Songdogwahak-ro, Yeonsu-Gu, Incheon 406-840, Republic of Korea
c
Ministry of National Defense, Seoul, Republic of Korea
d
Department of Architectural Engineering, Dankook University, Suji-Gu, Yongin 16890, Republic of Korea

h i g h l i g h t s

 Linear attenuation coefficient, l, of concrete was investigated.


 The l values of RCA are slightly lower than NCA.
 Surface dose rate of transportable concrete containers was examined.
 Maximum surface dose rate of the concrete containers was turned out below 2 mSv/h.

a r t i c l e i n f o a b s t r a c t

Article history: This paper presents an assessment of gamma radiation shielding performance, specifically in terms of
Received 20 July 2017 surface dose rate, of concrete containing virgin and recycled coarse aggregates (RCA) to be used for a
Received in revised form 17 November 2017 transportable concrete container for radioactive waste. In order to evaluate radiation shielding perfor-
Accepted 9 December 2017
mance of the transportable concrete container a numerical simulation method is performed using
Monte Carlo N-particle version 6.1 (MCNP6.1). Prior to evaluating radiation shielding performance of
the transportable concrete containers, radiation shielding properties of four different concrete mixtures
Keywords:
which have two different compressive strengths, 40 and 70 MPa, containing natural coarse aggregate
Recycled concrete aggregate
Gamma radiation shielding
(NCA) and recycled coarse aggregate (RCA), respectively, are assessed using experimental and numerical
Linear attenuation coefficient simulation methods in terms of linear attenuation coefficient (l) to verify the reliability of the numerical
Transportable container simulation method. Density, compressive strength, and static modulus of elasticity tests are conducted to
Radioactive waste determine the parameters for transportable concrete container design. Based on the physical properties
Surface dose rate of concrete a transportable concrete container is designed. In order to assess the radiation shielding with
MCNP6 respect to the maximum surface dose rate of the concrete containers, three different radioactive wastes
are assumed to be loaded in the containers with metal drums and radiation shielding analysis is carried
out using MCNP6 simulation code for the four different concrete containers, comparing with the existing
carbon steel container. It was found that the results from numerical simulation are in good agreement
with the experimentally determined results. In terms of the maximum surface dose rate, all concrete con-
tainers showed considerably lower surface dose rate than the existing carbon steel container.
Ó 2017 Elsevier Ltd. All rights reserved.

1. Introduction of the used fuels and with limited radioactive waste disposal space.
In order to be properly stored, this radioactive waste needs to be
One of the problems facing in nuclear industry is the accumula- transported in specific containers. The ideal container for radioac-
tion of radioactive waste from decommissioned nuclear power tive waste should meet rigorous criteria and the level of perfor-
plants; this is especially true for the countries with no reprocessing mance when handling and transporting. According to the
International Atomic Energy Agency (IAEA) regulations, there are
two primary considerations for the safe transport of radioactive
⇑ Corresponding author.
materials contained in any packaging [1]. The first consideration
E-mail addresses: dahee.han@utah.edu (D. Han), kimwj@poscoenc.com
(W. Kim), brain239@gmail.com (S. Lee), hykim00@dankook.ac.kr (H. Kim), romero@ is radiation protection in terms of surface dose rate limit and the
civil.utah.edu (P. Romero).

https://doi.org/10.1016/j.conbuildmat.2017.12.078
0950-0618/Ó 2017 Elsevier Ltd. All rights reserved.
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 123

second is physical soundness with respect to dropping and stack- mixtures is evaluated using experimental and numerical simula-
ing resistances. tion methods.
Nowadays, concrete is widely used as a shielding material Based on the physical properties of the concretes, a trans-
against radiation of strong penetrating power due to its effective portable concrete container for radioactive waste was designed
shielding characteristics, relatively low cost, and sufficiently long with respect to reinforcement based on the American Association
durability. For these reasons, many studies have been conducted of State Highway and Transportation Officials Load and Resistance
in assessing radiation shielding characteristics of hardened Factor Design (AASHTO LRFD) for culverts [15]. Furthermore, in
cement paste using various supplementary cementitious materi- order to assess the radiation shielding with respect to the maxi-
als such as ground granulated blast-furnace slag, fly ash, and sil- mum surface dose rate of the transportable concrete containers
ica fume and so on and of concrete using different kinds of three different radioactive wastes (a low and two intermediate
aggregates for several decades [2–7]. Meanwhile, one of the most levels), specially for gamma rays, are adopted to be loaded in the
important issues in construction industry is the depletion of vir- containers with metal drums and radiation shielding analysis is
gin aggregate and increase of concrete demolition waste. As part carried out using MCNP6 simulation code for the four different
of viable solution for those, use of recycled aggregates from con- concrete containers, comparing with the existing carbon steel
crete demolition waste was suggested. In this regard, many stud- container.
ies on mechanical properties and durable performance of
concrete containing recycled aggregates have been conducted 2. Materials
and shown a significant possibility to be used as structural mate-
rials [8–14]. However, there are very few studies dealing with Concrete with two different compressive strengths, 40 and 70
radiation shielding properties of concrete containing recycled MPa are analyzed in this study. For each concrete mixture, 100%
coarse aggregates (RCA). of crushed natural granite coarse aggregate (NCA) and recycled
The purpose of this study is to present the radiation shielding coarse aggregate (RCA), which is obtained from demolition build-
properties of transportable concrete containers made with RCA ings meeting Korean Standard F 2573 (KS F 2573) [16] are used.
and intended for transport of radioactive waste from decommis- The same type of sea sand is used as a fine aggregate (FA) for all
sioned nuclear power plants. This is done using a numerical simu- samples. Table 1 summarizes the properties of NCA, RCA, and FA,
lation code. Prior to evaluating the radiation shielding performance including the contents of KS F 2573 for recycled coarse aggregates.
of the transportable concrete containers, the physical properties of Ordinary Portland cement (OPC) equivalent to KS L 5201 Type 1
hardened concrete samples such as density, compressive strength, [16], ground granulated blast furnace slag (GGBFS) produced in
and static modulus of elasticity for two different compressive Gwangyang, South Korea, and silica fume (SF) manufactured in
strengths, 40 and 70 MPa, each made with 0% (considered the con- Canada are used as cementitious materials. Also polycarboxylate
trol sample) or 100% of recycled coarse aggregates are investigated. ether superplasticizer (SP) is added as an admixture. Table 2 shows
In total, radiation shielding performance of four different concrete chemical and physical properties of all of these materials except

Table 1
Properties of NCA (natural granite coarse aggregate), RCA (recycled coarse aggregate), and FA (fine aggregate).

NCA RCA KS F 2573 FA


Max. size (mm) 19 – 5
OD density (g/cm3) 2.62 2.49 Above 2.5 2.54
Absorption (%) 1.22 3.07 Below 3.0 1.44
Abrasion resistance (%) 17.4 25.9 Below 40 –
Soundness (%) 8.7 13.5 Below 12 4.1

Table 2
Chemical and physical properties of concrete mixture materials.

Weight fraction (%)


OPC (Type1) GGBFS SF XRF
FA NCA RCA
SiO2 21.10 35.18 96.50 91.76 74.60 56.54
Fe2O3 2.90 2.85 0.09 0.39 1.89 6.75
CaO 62.50 36.75 0.2 2.31 4.14 12.56
Al2O3 6.10 17.23 0.25 4.17 11.60 14.29
MgO 2.20 2.43 0.55 0.71 0.55 2.25
Na2O – 2.97 0.25 0.16 1.60 1.67
K2O 1.74 0.38 0.45 0.12 3.51 4.28
TiO2 – 0.97 – 0.11 0.60 0.75
P2O5 – 0.22 – 0.16 0.17 0.13
MnO – 0.37 – – 0.12 0.31
SO3 2.20 0.37 – – – 0.30
Others – 0.27 0.29 0.11 0.10 0.16
LOI 1.07 0.32 1.42 – – –
SG* 3.15 2.85 2.25 – – –
*
SG: Specific Gravity, OPC: Ordinary Portland Cement, GGBFS: Ground Granulated Blast Furnace Salg, SF: Silica Fume, FA: Fine Aggregate, NCA: Natural granite Coarse
Aggregate, RCA: Recycled Coarse Aggregate.
124 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

Table 3
Proportion of concrete mixtures.

W/B (%) S/a Unit weight (kg/m3)


Water Cement GGBFS SF FA NCA RCA SP (%)
40NCA 36.8 46.7 165 269 179 – 798 945 – 0.75
40RCA – 894
70NCA 22.6 40 160 389 283 35 593 824 – 2.65
70RCA – 778

W/B: Water-to-Binders ratio; S/a: Fine-to-coarse aggregate ratio; Weight of SP: Binders’ weight  SP (%).

Table 4
Elemental composition of each concrete mixture.

Elemental composition
Element Weight (%)
40NCA 40RCA 70NCA 70RCA
H 0.78 0.78 0.75 0.75
O 50.27 48.93 48.67 47.40
Na 0.83 0.70 0.9 0.78
Mg 0.40 0.94 0.52 1.04
Al 4.09 4.66 4.46 5.00
Si 31.12 27.81 27.97 24.78
P 0.07 0.06 0.07 0.06
S 0.11 0.06 0.17 0.06
K 1.41 1.65 1.45 1.66
Ca 8.08 10.48 12.26 14.53
Ti 0.21 0.25 0.22 0.26
Mn 0.06 0.06 0.07 0.07
Fe 1.11 2.09 1.17 2.45

the admixture. Table 3 provides the data on the proportion of the strength at 3, 7, and 28 days of curing. In order to perform the com-
concrete mixtures used in this study. The chemical compositions pressive test, a cylinder is placed in the center of a pressure plate,
of NCA, RCA, and FA are determined using X-ray Fluorescence and load is applied at a rate of 0.6 ± 0.4 MPa/s. The load is increased
(XRF) method and the values are provided in Table 2; chemical for each sample until it fails. Three cylinders per concrete mixture
properties of other ingredients used in concrete mixes are provided are tested and the average value of three concrete samples is
from each manufacturer. Table 4 shows the elemental composition reported. The final compressive strength of all concrete mixtures
by fraction weight for each concrete mixture. is compared to the design strengths at a curing age of 28 days as
specified in ASTM C192 [17].
3. Physical properties of concrete
3.3. Static modulus of elasticity and Poisson’s ratio
3.1. Density of hardened concrete
The Young’s modulus of elasticity of the concretes is deter-
mined using the standard methods for static modulus of elasticity
The chemical composition of concrete has an important effect
and Poisson’s ratio of concrete in compression based on ASTM
on its radiation shielding properties. The density of concrete is also
C469 [18]. Three cylindrical specimens of 100 mm in diameter
of importance for shielding against gamma rays, with denser mate-
and 200 mm in height are used for each concrete mixture and
rial exhibiting better shielding properties than porous one. For
the average values are reported.
these reasons, a density test of hardened concrete is conducted.
The samples size is 100 mm in diameter and 200 mm in height.
The samples are cured for 91 days in a chamber room at a temper- 3.4. Results of physical properties of concrete
ature of 20 ± 5 °C and air relative humidity of 50 ± 10%. The atmo-
spheric curing density (ACD) of a sample is determined using Eq. 3.4.1. Density of hardened concrete
(1). Fig. 1 shows the ACD density for each of the concrete samples; it
can be seen that the densities range from 2.289 to 2.398 (g/cm3).
 g   wACD

The RCA samples show slightly lower density when compared to
ACD density ¼  100 ð1Þ
cm3 ðwACD  ww Þ NCA samples. The lower density of the RCA mixtures is in agree-
ment with other studies [19,20]; it is attributed to the lower den-
where WACD represents a mass of atmospherically cured sample, Ww sity of RCA.
is a mass of atmospherically cured sample in water, and q is a den-
sity of water. 3.4.2. Compressive strength
The results of the compressive strength tests for each concrete
3.2. Compressive strength mixture are shown in Fig. 2. As can be seen in Fig. 2, the design
compressive strength of all concrete mixtures is achieved at the
Cylindrical samples, with the same size used for density tests, 28th day. The compressive strength of RCA samples for both 40
are cast in steel molds and kept in a mist room at 20 ± 3 °C for and 70 MPa is lower than those obtained for the NCA samples. In
24 h until demolding. Once demolded, cylinders are placed in a more detail, the compressive strengths for 40RCA samples at 28
water bath at temperature of 25 ± 2 °C and tested for compressive curing days are 11% lower than 40NCA samples. Also, the compres-
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 125

2.6 4. The linear attenuation coefficients of concrete


2.398
2.4 2.308 2.289 2.321
4.1. Experimental method for assessing radiation shielding properties
2.2
of concrete
ACD Density (g/cm3)

1.8
For each mixture, cylindrical concrete samples are cut into sam-
ples of 100 mm in length and used for radiation shielding test. A
1.6 Cs-137 source of 1.79 lCi strength, (emitting gammas of energy
1.4 0.6617 MeV) is used as a gamma source. It is well known that Lan-
thanum Bromide (LaBr3) scintillation detectors offer significantly
1.2
better resolution and higher efficiency than sodium iodide (NaI)
1 scintillation detector [22]. Therefore, LaBr3 scintillation detector
40NCA 40RCA 70NCA 70RCA
is used to measure the gamma energy spectrum with concrete
Type of Sample
sample and without concrete sample. The geometry of the experi-
Fig. 1. Density of concrete samples (with compositions defined in Table 4). mental test setup is shown in Fig. 4. The Cs-137 source and con-
crete samples are placed on a holder. This arrangement allows
the radioactive source and concrete samples to remain in contact
90 during the experiment. A detector is suspended above the concrete
sample using a detector holder. The experimental measurements
Compressive Strength (MPa)

80
70 are taken twice for each sample. First, a radiation count reading
is taken without a concrete sample, indicating the intensity of
60
the source (I0). The following measurement includes the concrete
50
sample, thus indicating transmitted intensity (I) of gamma radia-
40 tion. For each concrete sample, the measurement is repeated three
30 times and the average peak value is used to calculate a linear atten-
20 uation coefficient. Based on these values I0 and I, a linear attenua-
40NCA 40RCA
10 70NCA 70RCA tion coefficient (l) is calculated using Beer-Lambert law defined in
Design strength (40MPa) Design strength (70MPa) Eq. (2).
0
0 7 14 21 28 1
Age (days) I ¼ I0 elx ! l ¼ ðlnI0  lnIÞ ð2Þ
x
Fig. 2. Compressive strength of each concrete mixture.
where x is thickness of a concrete sample.
The elemental composition of concrete affects its radiation
sive strengths for 70RCA samples at 28 curing days are 8% lower shielding properties because different elements interact with
than 70NCA samples. This can be attributed to relatively poor gamma rays of a given energy differently [23]. For composite mate-
interfacial transition zone between cement matrix and RCA [21]. rials such as concrete, the linear attenuation coefficient (l, cm1)
can be obtained from the total mass attenuation coefficient (lq)
as described in Eq. (3).
3.4.3. Young’s elastic modulus and Poisson’s ratio
 
The Young’s elastic modulus determines the resistance of any l X l
¼ wi ð3Þ
material to elastic deformation when a force is applied to the q i
q i
material. It is an essential parameter for reinforced concrete struc-
tural design. Fig. 3 shows the results of the Young’s elastic modulus where Wi and (l/q)i are the fraction by weight and mass attenua-
and Poisson’s ratio for all concrete specimens. As can be seen in tion coefficient of ith component, respectively.
Fig. 3, the elastic moduli of 40NCA and RCA are 37.21 and 32.32
GPa respectively. For 70 MPa series, NCA and RCA show 44.82 4.2. Numerical simulation method
and 37.90 GPa, respectively. Poisson’s ratio values range from
0.175 to 0.204 although no trend is observed. The particle radiation transport code, MCNP (Monte Carlo N-
Particle), is used to simulate the transport of 37 different particle
types for reactor criticality, shielding, dosimetry, detector
55 0.25
Elastic modulus (Ec) Poisson's ratio (v) response, and many other applications [24]. In this study, MCNP6
50
code is used to determine linear attenuation coefficients of con-
Young's elastic modlus (GPa)

45 0.2 crete mixtures. In MCNP6 models, the elemental compositions


40 shown in Table 4 are used in material cards. The geometry of all
Poisson's ratio

35
0.15 parameters is set up in accordance with the actual experiment.
30 Radioactive source is defined as a degenerate cylindrical volume
25 source; a circle lies in a plane perpendicular to an axis at a given
0.1 distance, which is equivalent to the actual source used in the
20
15 experiment. Fig. 5 shows the particle tracks emitting from the
10 0.05 source. The LaBr3 detector is defined as a detector and designated
to record data using the F8 tally. In order to determine a linear
5
attenuation coefficient of each concrete mixture, the simulation
0 0
40NCA 40RCA 70NCA 70RCA
is executed twice with 1,00,00,000 histories. These provide the
Type of concrete intensity values without and with concrete to be recorded and then
employed as I0 and I. MCNP6 is based on Monte Carlo method to
Fig. 3. Elastic modulus and Poisson’s ratio. simulate particle transport such as neutrons, electrons, and
126 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

LaBr3
detector

Φ : 100 mm

x : 100 mm Concrete
sample

Cs137 source

Holders

a) With concrete sample b) Without concrete sample


Fig. 4. Experimental setup.

LaBr3
detector

Cs-137
source

Source
Holder
Fig. 5. MCNP6 model of the gamma rays tracks emitted from the Cs 137 source.

photons with continuous-energy, generalized geometry, and time- keV to 100 GeV [26]. In this study, Xcom is used to obtain a linear
dependent [25], while Xcom (photon cross sections database) is attenuation coefficient of each concrete mixture. The elemental
based on deterministic method with theoretical data, providing compositions presented in Table 4 are used in Xcom to determine
photon cross sections for scattering, photoelectric absorption and the total mass attenuation coefficients and then the linear attenu-
pair production, as well as total attenuation coefficients for various ation coefficients that are obtained by multiplying density of each
mixtures with 100 of atomic numbers at energies ranging from 1 concrete sample. In the last step, the linear attenuation coefficients
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 127

obtained from Xcom and MCNP6 code are compared with the val- case without concrete samples (Figs. 4 and 5) show much higher
ues from the experiments. values compared to the case with concrete samples. This indicates
that gamma rays are attenuated by concrete sample. The normal-
4.3. Error propagation ized transmission rates in the experiment range from 0.1574 to
0.1786 for all concrete mixtures. From the MCNP6 simulation it
The number of counts reading in an experiment tends to follow can be seen that the normalized transmission rates range from
a Gaussian distribution. Meanwhile, the MCNP6 outputs provide 0.156 to 0.168, which is in good agreement with the experimental
relative errors, for both rI and rI0, of the peak at certain energy. values.
Based on these, standard errors of the linear attenuation coefficient Based on the I and I0 values obtained from both the experimen-
obtained from the experimental measurements are determined as tal measurements and MCNP6 simulation for all concrete samples,
shown in Eq. (4). the total mass attenuation coefficients are calculated and com-
sffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi pared with Xcom data, as shown in Fig. 7. In comparison of the
 2  2
@l @l total mass attenuation coefficients obtained from the experimental
rl ¼ r2I þ r2I0 ð4Þ
@I @I0 method to the results from numerical simulation MCNP6 and
Xcom, the results from both numerical simulation and Xcom range
where l is the linear attenuation coefficient, I is transmitted inten- within 5 percent of error amount, implying that there is a good
sity, I0 is unshielded intensity, and rI and rI0 are standard errors of agreement between the experimentally measured and numerically
transmitted intensity and unshielded intensity respectively. In simulated mass attenuation coefficients. In addition, it is obvious
addition, for errors of the numerical simulation, the relative errors that the experimentally determined total mass attenuation coeffi-
provided by MCNP6 simulation are utilized. cients are slightly lower than the results obtained from MCNP6 and
Xcom. This might be attributed to the crystalline nature of the
4.4. Results of the linear attenuation coefficients of concretes molecular arrangement of detector source which can make inci-
dent beam geometry narrow, possibly reducing the total mass
Both, the NCA and RCA samples are tested for their linear atten- attenuation coefficient values [25,28].
uation coefficients for the two different design compressive The linear attenuation coefficient values with the errors are pro-
strengths (40 and 70 MPa). Fig. 6 displays the gamma energy spec- vided in Table 6. The standard errors of experimentally determined
tra obtained from Cs-137 source with concrete samples and with- linear attenuation coefficients for each concrete mixture range
out concrete samples. As can be seen in Fig. 6, the peak number of from ±0.0154 to ±0.0165, indicating that all measurements are
counts is shown at 0.6617 MeV of gamma energy, following a Pois- within 2rl, 95% confidence interval. The relative errors obtained
son distribution under the explicit assumption that the Poisson from the MCNP6 models range from ±0.0332 to ±0.0344 which is
distribution can be approximated by a Gaussian distribution. How- considered as low error [24]. When linear attenuation coefficient
ever, it should be noted that if the number of counts increases of 40RCA is compared to 40NCA, no significant differences are
enough, the Gaussian approximation is not valid [27]. Table 5 found. However, for 70 MPa series, RCA samples show slightly
shows the average transmission values obtained from the experi- lower linear attenuation coefficients than NCA. This can be attrib-
ment and MCNP6 simulation. Aforementioned above, these values uted to lower density rather than the chemical properties. This is
correspond to the gamma energy of 0.6617 MeV; the values are because the total mass attenuation coefficient of 70RCA is close
normalized to unity. As it can be seen in Table 5, both the experi- to 70NCA.
mental average number of counts and MCNP6 probabilities for the
0.09 Exp. MCNP6 Xcom Error amount: 5%
2/g)

350 Without concrete 40 NCA


40 RCA 70 NCA 0.08
300 70 RCA
250
0.07
200
Counts

150

100 0.06

50

0 0.05
0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 40NCA 40RCA 70NCA 70RCA
Photon Energy (MeV) Type of concrete sample

Fig. 6. Gamma energy spectra obtained from Cs-137 source with concrete and Fig. 7. Measured and numerically determined total mass attenuation coefficients
without concrete samples. for each concrete sample.

Table 5
Experimental and MCNP6 values for various concrete mixtures.

Without concrete sample (I0) With concrete sample (I)


40NCA 40RCA 70NCA 70RCA
Exp. Counts 281.67 48.33 50.33 44.33 49.33
Normalized 1 0.1716 0.1786 0.1574 0.1751
7
MCNP6 (1  10 particles) Probability 5.41E04 9.09E05 9.23E05 8.44E05 9.02E05
Normalized 1 0.1680 0.1706 0.1560 0.1667
128 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

5. Radiation shielding properties of transportable concrete ing and storing radioactive materials. In this section, based on the
containers IAEA regulations [1], an IP-2 type concrete container is designed
and assessed with respect to radiation shielding performance, then
5.1. Reinforcement design of containers compared to the existing IP-2 type steel container. The shape and
size of the IP-2 type concrete container is referred from the existing
In design of packaging to transport radioactive material, two IP-2 type steel container. The dimensional properties of both con-
main aspects should be complied with IAEA regulations [1]. The tainers are shown in Fig. 8.
first is associated with radiation shielding performance in terms Based on the dimensional properties of the concrete container,
of surface dose rate limit. The other one is related to physical structural analysis to design reinforcement of concrete container is
soundness such as resistance to free drop and stack for transport- investigated. AASHTO LRFD bridge design specifications for culvert
were referred [15]. The approximate strip method is used for the
design with 1 foot (30 cm) wide design strip. A 3-Dimensional shell
Table 6 frame model is used to analyze the container. The material and
Linear attenuation coefficients values with errors of each concrete sample. design parameters are shown in Table 7. In order to analyze the
structural properties of concrete containers, applicable load combi-
Concrete sample ACD Linear attenuation coefficient
density (l, cm1) at 0.6617 MeV nations and load factors are selected as shown in Table 8. Based on
(g/cm3) the load combinations and factors, a structural analysis is per-
Exp. ± Standard MCNP6 ± Relative
errors errors
formed using a commercial matrix analysis program. Table 9
shows the structural analysis result.
40NCA 2.308 0.1763 ± 0.0156 0.1784 ± 0.0332
40RCA 2.289 0.1723 ± 0.0154 0.1769 ± 0.0329
Eventually, the areas and spacing of steel reinforcement for
70NCA 2.398 0.1849 ± 0.0165 0.1858 ± 0.0344 each member are determined by strength limit state for flexure
70RCA 2.321 0.1743 ± 0.0155 0.1792 ± 0.0333 in accordance with AASHTO LRFD design specifications and crack
control, shear limit, minimum reinforcement limit, and maximum

3304

3280
12 274.6 570 150.25 570 150.25 570 150.25 570 274.6 12

91 12
570

1480

1504
158
570
12 91

3400
1200

a) Inner and external dimensions of the existing carbon steel container


Fig. 8. Dimensions of the existing and concrete container (unit: millimeter, mm).
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 129

150

570

1300 1600
100

80
52
150

150 2720 150

3020

180

840 1200

180

b) Inner and external dimensions of concrete containers


Fig. 8 (continued)

Table 7
Materials and design parameters.

Unit weight Reinforced concrete, cc 2400 kg/m3


Concrete Compressive Strength, f’c 40 MPa (6 ksi), 70 MPa
Lid thickness, TL 0.18 m
Bottom slab, Tb 0.18 m
Wall thickness, Tw 0.15 m
Reinforcement clear cover 0.04 m
Modulus of elasticity, Ec 33 GPa
Steel reinforcement Modulus of elasticity, Es 200 GPa
Yield strength, fy 400 MPa
Reinforcement bar D13 (12.7 mm, D, 126.7 mm2, A)
Maximum rebar spacing Wall 200 mm (8 in) longitudinal
250 mm (10 in) transverse
Lid and slab 200 mm (8 in) longitudinal
250 mm (10 in) transverse

reinforcement limit are checked, satisfying with the specifications. code for four different concrete mixtures, comparing to the existing
Fig. 9 shows the final reinforcement design of concrete container. carbon steel container manufactured by Korea Hydro & Nuclear
Power co., Ltd. (KHNP) [29].

5.2. Evaluation of surface dose rate limit


5.2.1. Description of numerical simulation analysis
In order to assess the radiation shielding integrity of packages Radioactive waste consists of various kinds of radionuclide that
in terms of surface dose rate of the concrete containers containing emits different radiations such as alpha, beta particles, and gamma
low and intermediate level of radioactive waste, respectively, radi- rays. In this study, for radioactive waste source three different
ation shielding analysis is carried out using MCNP6 simulation types of radioactive waste source terms are used, neutron activated
130 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

Table 8
Applicable load combinations and factors.

Dead load (DL) Top lid 0.18 m  1.60 m  3.02 m  2400 kg/m3 = 2087 kg
Long wall (0.15 m  0.84 m  3.02 m  2400 kg/m3)  2 = 1826 kg
Short wall [0.15 m  0.84 m  (1.6–0.3)  2400 kg/m3]  2 = 786 kg
Bottom slab 0.18 m  1.6 m  3.02 m  2400 kg/m3 = 2087 kg
Total DL 2087 + 1826+786 + 2087 = 6786 kg
Live load (LL) - Assumption: two more packages are stacked on the very bottom package
(1) Eight of 200 L drums with maximum weight of 480 kg; 8  480 kg  2
packages = 7680 kg
(2) Weight of two containers; (2087 + 1826 + 786 + 2087)  2 = 13,572 kg
(3) Eight of 200 L drums on the bottom slab of very bottom package; 8  480 kg
= 3840 kg
- Total live load
7680 + 13,572 + 3840 = 25,092 kg
Load combos Strength limit state 1.25DL + 1.75 LL
Service limit state 1.0DL + 1.0 LL

Table 9
Structural analysis results for load combinations.

Top lid Long side wall Short side wall Bottom slab
Inside Outside Inside Outside
Strength Max. moment (kN-m) 5.70 2.11 5.34 0.62 2.26 1.72
Governing shear (MPa) 47.61 12.55 7.65 13.31
Associated Mu (kN-m) 0.20 0.47 0.16 0.01
Service Max. moment (kN-m) 3.32 1.22 3.12 0.36 1.32 1.05
Governing shear (MPa) 27.17 7.38 4.48 8.20

A A'

1600

3020

180

D13 @ 200 D13 @ 250 D13 @ 200

D13 @ 250

840 1200

D13 @ 250 D13 @ 200

180

Fig. 9. Reinforcement design of concrete container (unit: millimeter, mm).


D. Han et al. / Construction and Building Materials 163 (2018) 122–138 131

Table 10
Physical and chemical properties of A533B alloy steel.

Chemical compositions (wt%)


C Al Si P S V Cr Mn Fe Ni Cu Mo
0.18 0.014 0.24 0.017 0.004 0.002 0.12 1.42 Bal. 0.84 0.14 0.51
Density
7.874 g/cm3

Table 11
Physical and chemical properties of biological shielding concrete.

Chemical compositions (Weight fraction)


H C O Na Mg Al Si K Ca Fe
0.0221 0.00248 0.5749 0.01521 0.0013 0.01995 0.30463 0.01005 0.04295 0.00644
Density
2.300 g/cm3

Table 12
Activity inventory of RPV and biological shielding concrete of the designated reactors.

Component Nuclides Half-life (year) Specific activity* (Bq/g) Fraction (%)


4
WWER-440 RPV Mn-54 0.83 1.80  10 0.656
Fe-55 2.74 2.47  106 88.677
Co-60 5.30 2.90  105 10.412
Ni-59 7.60  104 7.40  101 0.003
Ni-63 1.00  102 7.30  103 0.262
Total 2.79  106 100.000
Biological shielding concrete of WWER-440 Ca-41 1.00  105 1.12  100 0.011
Co-60 5.30 7.50  101 0.751
Eu-152 13.50 9.48  103 94.938
Eu-154 8.60 4.20  102 4.206
Cs-134 2.50 8.12  100 0.081
Fe-55 2.74 1.22  100 0.012
Mn-54 0.83 1.11  100 0.011
Total 1.85  104 100.00
AM RPV Mn-54 0.83 1.32  104 0.014
Fe-55 2.74 7.50  107 78.140
Co-60 5.3 9.10  106 20.837
Ni-59 7.60  104 8.20  103 0.009
Ni-63 1.0  102 9.60  105 1.000
Total 9.60  107 100.000
*
10 years elapsed after final shutdown.

activity inventories of the reactor pressure vessel (RPV) and biolog- In addition, it is essential to classify the different kinds of
ical shielding concrete of the Water-Water Energetic Reactor-440 radioactive waste for managing them more effectively. Therefore,
(WWER-440) type operated in Armenia [30], and the activity based on the specific activity values in Table 12, radioactive waste
inventory of the reactor vessel of the Russian Atom Mirny (AM) from WWER-440 and AM RPV are classified using Eq. (5).
reactor type operated in Obninsk, Russia [31]. The RPV of
WWER-440 and AM reactor were made of A533B alloy steel pro- X
n
TACi
¼ WCI ð5Þ
duced using the basic oxygen furnace-ladle refining furnace i¼1
EACi
(BOF-LRF) process. For the biological concrete of WWER-440 nor-
mal concrete was used. Tables 10 and 11 show the chemical and where WCI is waste classification index, n is the number of radionu-
physical properties of A533B alloy steel and biological shielding clides, TACi is the total activity of ith radionuclide, and EACi is the
concrete respectively. activity concentration for exempt material, also known as clearance
Such reactor parts exposed to neutron radiation around reactor level, of ith radionuclide. As can be seen in Eq. (5), the WCI values
core contain elements that can be transformed into radionuclides imply where the radioactive waste should be classified. If the WCI
that emit radiation. Radioactive waste is mainly classified by type is equal to or less than 1.0  103 the radioactive waste can be con-
of radionuclides, their concentrations, and half-life. The regulations sidered as low level radioactive waste, if WCI values ranged from
of IAEA [1] provide sufficient information on the limit and basic 1.0  103 to 1.0  106, it can be considered as intermediate level
radionuclide values which should be concerned. Based on the reg- radioactive waste. Lastly, if WCI values exceed 1.0  106, the
ulations, the radioactivity concentration in specific activity and radioactive waste should be classified as high level radioactive
half-life of the principal radionuclides of the RPV of WWER-440, waste [30]. In addition, for the activity concentration for exempt
AM reactors, and biological shielding concrete of WWER-440 ana- materials also known as exemption or clearance level, even though
lyzed by Babcsány et al. and Suvorov et al. [30,31] are shown in EAC values differ from each country regulation, EAC values in this
Table 12. study are referred from IAEA (2009) [1] to calculate WCI. Table 13
132 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

shows the EAC values for the principal radionuclides of the three Radioactive waste sources in the drums, containing only gamma-
components. rays emitting radionuclides, are assumed to be homogenized and
Based on the specific activities and EAC values in Tables 12 and evenly distributed inside the drums. For the geometrical properties
13, WCI of RPV of WWER-440 and AM reactors and biological of the existing IP-2 type developed by KHNP, the geometry of all
shielding concrete of WWER-440 is calculated by using Eq. (5) parameters shown in Fig. 7 is modeled by using the geometry spec-
and classified as each level. Fig. 10 shows the calculated WCI val- ifications. However, in a regard of the worst scenario, namely for
ues of each component. conservative analysis for shielding performance of the IP-2 type
As can be seen in Fig. 9, WCI values of WWER-440 RPV and AM KHNP container, reinforced channels on the side walls and lifting
RPV component were 3.10E+4 and 9.19E+5 respectively. Since the attachments are excluded, only modeling the thinnest walls. For
values range between low and intermediate level, they can be con- radioactive waste sources and drums, all parameters are modeled
sidered as intermediate level radioactive waste. In addition, WCI in the same way for the IP-2 type concrete container. Fig. 11 shows
value of biological shielding concrete for WWER-440 reactor was the geometrical properties of the both IP-2 type containers created
9.98E+2, which is below 1.00E+3. Therefore, biological shielding by MCNP visual editor on 3-D dynamic plotting.
concrete for WWER-440 can be considered as low level radioactive
waste.
5.2.3. Numerical simulation details on input cards
In order to evaluate radiation shielding performance using
5.2.2. Geometrical properties of numerical simulation numerical simulation program, it is essential to define data cards
MCNP6 is executed based on geometrical properties of a model set such as source, material, and tally cards. For material cards,
so the results obtained from the simulation are significantly the drums and IP-2 type KHNP container are defined as carbon
affected by the geometrical properties. Therefore, an exact and rea- steel and their elemental compositions and physical properties
sonable geometrical setup for model is one of the most essential are shown in Table 14.
concerns on executing MCNP6. In order to evaluate the radiation Four different concrete mixtures are used for IP-2 type concrete
shielding performance of IP-2 type concrete container designed container. In other words, a numerical simulation for each concrete
in this study and the existing IP-2 type steel container developed mixture is performed. The elemental components of each concrete
by KHNP, radiation shielding analyses in terms of surface dose rate mixture are shown in Table 4. For radioactive source, multiple arbi-
limit are performed using MCNP 6.1 V. For geometrical properties trary volumetric sources with different energy photons in the form
of IP-2 type concrete container, the geometry of all parameters of a cylinder filled into the steel drums are defined in radioactive
shown in Fig. 8 is modeled by using the geometry specifications source cards. This method uses the rejection technique by setting
of MCNP 6.1 V. In addition, eight 200-liter drums are loaded in a finite room over designated source cells. In this method, size
the container and all drums are identically modeled with a diame- and location of the designated source cells and source photon ener-
ter of 570 mm, height of 850 mm, and thickness of 1.2 mm. gies play a main role in defining source specifications. The source
photon energies of the principal radionuclides of the RPV of
Table 13 WWER-440 and AM reactors and biological shielding concrete of
The EAC values for the principal radionuclides of the RPV of WWER-440 and AM
WWER-440, shown in Table 12, are defined in source cards respec-
reactors and biological shielding concrete of WWER-440.
tively. Table 15 shows the source photon energies of the nuclides
Principal Nuclides Half-life (year) Activity concentration obtained from RPV of WWER-440 and AM reactors and biological
for exempt material (Bq/g)
shielding concrete of WWER-440.
Mn-54 0.83 1  101 Flux tally at a point, also known as F5 type, is defined in the tally
Fe-55 2.74 1  104
card. Using the coordinates of the point detector, the flux values in
Co-60 5.30 1  101
Ni-59 7.60  104 1  104 unit of the number of particles per cm2 are measured on the sur-
Ni-63 1.00  102 1  105 face of the IP-2 type containers. Therefore, the point detectors
Ca-41 1.00  105 1  105 are defined to be placed on the sides and top of the containers.
Eu-152 13.50 1  101 Fig. 12 shows all points where the flux is measured. For particle
Eu-154 8.60 1  101
transport history, in order to decrease uncertainty in regard to
Cs-134 2.50 1  101
the tally results the number of particles is defined up to 1E+07.

WCI Low level limit(1E+3) Intermediate level limit(1E+6)


Waste classification Index

1.0E+07
1.0E+06 9.19E+05
1.0E+05 3.10E+04
1.0E+04
9.98E+02
1.0E+03
1.0E+02
1.0E+01
1.0E+00
WWER-440 RPV
WWER-440
AM RPV
concrete
Fig. 10. WCI values of WWER-440 and AM RPV and WWER-440 concrete structure.
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 133

conversion factors using MCNPX code at the decommissioning


stage of Ignalina nuclear power plant [37]. The results showed that
the data obtained from the ANSI/ANS-6.1.1-1991 were the most
reliable for various doses and shielding calculations in the case of
decontamination of radioactive equipment and similar applica-
tions, turning out a statistically good agreement between the sim-
ulation results and experimental results. Therefore, in this study
the flux-to-dose conversion factors from ANSI/ANS-6.1.1-1991
are used to determine the dose rate. ANSI/ANS-6.1.1-1991 stan-
dard is based on and nearly identical to the photon sets in ICRP-
51 [33]. This standard presents data recommended for computing
the biologically relevant dosimetric quantity in gamma-ray radia-
a) IP-2 type concrete container with drums
tion fields. Specifically, this standard is intended for calculating
effective dose equivalent by shielding. Gamma-ray energies from
0.01 to 15 MeV are taken into account for effective dose equivalent
per unit fluence. Meanwhile, in order to determine flux-to-dose
rate at any energy point between 0.01 and 15 MeV with respect
to the conversion factor of ASNI/ANS-6.1.1-1991, the photon
energy rage is divided into four energy groups, 0.01–0.03, 0.03–
0.5, 0.5–5.0, and 5.0–15.0 MeV. For each energy group, regression
fitting is conducted until meeting the goal coefficient of determina-
tion, R2 of 0.999. A quartic regression fit met the goal coefficient of
determination as can be seen in Table 16. The general form of the
analytic function is the following Eq. (6).
b) IP-2 type KHNP container with drums

Fig. 11. Scheme of concrete and KHNP IP-2 type containers. 4 þbx3 þcx2 þdxþC
CF n ¼ eax ð6Þ

where CFn is flux-to-dose rate factors in (rem/h)/(photon/cm2s) and


5.2.4. Flux-to-dose rate convert factors x is ln(E) (E: Gamma-ray energy in MeV). The coefficients (a, b, c,
From the point of view of environmental radiological assess- and d) and constant number (C) obtained from the regression fitting
ments, the most important problem in external dosimetry is to are shown in Table 16. Based on the above, the conversion factors
estimate the dose to an individual or population due to exposure for photon energies between 0.01 and 15 MeV can be computed
to any radiations emitted by radionuclides. In general, it is difficult using the analytic equation, Eq. (6). In addition, this analytic form
to obtain realistic estimates of external dose from arbitrary distri- can be useful for the calculation of energy-averaged dose rates [38].
butions of radionuclides in the environment. Therefore, it is often Finally, based on the values of the flux obtained from MCNP6
assumed that exposure conditions are simplified and idealized; tally, flux-to-dose-rate above, and radioactivity shown in Table 12,
namely, that the distribution of sources at any location in the envi- the surface dose rate of sixteen different concrete containers and
ronment is effectively infinite or semi-infinite in extent and the
radionuclides concentrations or activities are uniform throughout
the source region [32], In addition, it is often assumed that the only
shielding between the radioactive sources and the body surface of Table 15
Photon energies of the primary nuclides obtained from RPV of WWER-440 and AM
the exposed individuals is provided by the medium through which
reactors and biological shielding concrete of WWER-440.
the radiations are transmitted. Thus, no accounting is made for
shielding provided by buildings during indoor residence, by cloth- Principal nuclides Half-life (year) Photon energy (Gamma-ray)
ing, or by buildings and irregular terrain during outdoor exposures. [MeV (frequency %)]

In order to improve the conservative dose limitation systems, Mn-54 0.83 0.834 (99.9)
many studies have been conducted to improve the system in terms Fe-55 2.74 0.006 (16.6)
Co-60 5.30 1.173 (100), 1.332 (100)
of flux-to-dose conversion factors for gamma-rays. Fig. 13 shows Ni-59 7.60  104 0.007 (20)
the four different flux-to-dose conversion factors obtained from Ni-63 1.00  102 0 (0)
American National Standards Institute (ANSI) and International Ca-41 1.00  105 0.003 (7.5)
Commission on Radiological Protection (ICRP) [33–36]. Eu-152 13.50 1.408 (21)
Eu-154 8.60 1.274 (35)
Stankunas et al. assessed and benchmarked the impact on
Cs-134 2.50 0.6 (98), 0.796 (85)
gamma dose rate employing four different photon-to-dose

Table 14
Physical and chemical properties of carbon steel for drums.

Chemical compositions (wt%)


C Si Mn Cr Ni S P Cu Fe
0.40 0.25 0.60 0.15 0.20 0.02 0.02 0.18 Bal.
Density
7.820 g/cm3
134 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

the existing container are calculated using Eq. (7). Gamma rays of In the same manner of the flux values obtained from MCNP6
Fe-55, Ni-59, Ni-63, and Ca-41 are not considered since numerical simulation, for both the existing KHNP and concrete
their energies are too low to be included in the range of the containers the maximum photon flux values are shown along
flux-to-dose-rate conversion factors. the center line of the radioactive sources on the surface of the
X and Y-plane. Meanwhile, the maximum photon flux values
  !  
mSv 1X n
mSv =h on the Z-plane of both types of containers are shown in the
Surface dose rate ¼ CF k  /mcnp  A  10 middle of the containers. Based on the photon flux values,
h n k¼1 rem=h
radioactivities, and flux-to-dose conversion factors, surface dose
ð7Þ rates of the both types of containers containing three different
where CFk is Flux-to-dose-rate conversion factors in (rem/h)/(pho- types of radioactive wastes, respectively are calculated using
ton/cm2s), Umcnp is Flux obtained from MCNP6 in #/cm2, and A is Eq. (7) above. Table 17 shows the maximum surface dose rates
Radioactivity in Bq (1Bq = 1 disintegration/s). on the X, Y, and Z-plane of the both existing KHNP and concrete
containers with three different types of radioactive waste. As can
be seen in Table 17, the maximum surface dose rate of the KHNP
5.3. Results of surface dose rate container loaded with AM RPV exceeds 2 mSv/h which is the sur-
face dose rate limit regulated by IAEA. On the other hand, the
In order to determine surface dose rate of the existing KHNP IP- maximum surface dose rates of all concrete containers with
2 type container and IP-2 type concrete containers designed in this AM RPV which is classified as intermediate level radioactive
study with respect to three different types of radioactive waste waste are less than the surface dose rate limit. For both
from decommissioned nuclear power plants MCNP6 numerical WWER-440 RPV and WWER-440 bioshielding concrete which
simulation is firstly performed to determine the flux on the exter- are classified as low and intermediate level radioactive waste
nal surfaces of the containers. Fig. 14 shows MCNP6 particle tracks respectively, the maximum surface dose rates of KHNP and all
displayed on the surface and tallies. As can be seen in Fig. 14, for concrete containers are significantly less than the surface dose
the both existing KHNP and concrete containers the highest num- rate limit.
ber of particles and their energy strength are shown in the middle Fig. 15 compares the maximum surface dose rate ratio of all
of drums on the surface of the X and Y-plane. In other words, the concrete containers to KHNP container. As seen in Fig. 15, for AM
maximum number of particles and energy are shown along the RPV the maximum surface dose rate ratios of concrete containers
center line of the radioactive sources. On the other hands, the max- to KHNP container ranged from 28.0 to 29.7% on the X-plane with
imum number of particles and energy on the Z-plane of both types an average of 28.8%, 26.4 to 31.3% on the Y-plane with an average
of containers are shown in the middle of the containers as can be of 28.9%, and 3.2 to 6.7% on the Z-plane with an average of 4.9%. For
seen in e) and f) of Fig. 14. WWER-440 RPV, the ratios are ranged from 36.4 to 40.0% on the

3304

27 50
27

50

1504
Z

X ZY
Y

ZX

1504 3304

27 50 23 50
23
27

895

895
50
50

YZ
Y XZ

a) IP-2 type KHNP container


Fig. 12. All points for measuring flux.
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 135

3020

150
150 50

50

1600
Z

Y X
ZY

ZX

1600 3020
180
180

150 50 150 50
1200

1200
YZ
50

Y XZ X

b) IP-2 type concrete container


Fig. 12 (continued)

1.E-04
Conversion factors [(rem/hr)/(p/cm2·Sec)]

1.E-05

1.E-06

ANSI/ANS-6.1.1-1977
1.E-07
ICRP-21
ANSI/ANS-6.1.1-1991
ICRP-74
1.E-08
0.01 0.1 1 10 100
Photon energy (MeV)
Fig. 13. Four different versions of dose conversion factors for photon.

Table 16
Polynomial coefficients for gamma-ray Flux-to-dose-rate conversion factors.

Photon Energy (MeV) a b c d C R2


0.01–0.03 – 3.3310E1 3.0043 9.3754 5.6393 1
0.03–0.5 8.740E2 7.6370E1 2.1450 1.3725 1.4082E1 0.9996
0.5–5.0 1.310E1 3.3690E1 2.1780E1 6.6820E1 1.3157E1 0.9995
5.0–15.0 – 1.200E2 1.7870E1 1.5300 1.2766E1 1
136 D. Han et al. / Construction and Building Materials 163 (2018) 122–138

a) X plane of KHNP container

b) X-plane of concrete container

c) Y-plane of KHNP container d) Y-plane of concrete containers

e) Z-plane of KHNP container

f) Z-plane of concrete containers


Fig. 14. MCNP6 particle tracks.

X-plane with an average of 38.2%, 42.5 to 45.1% on the Y-plane ratios are ranged from 10.0 to 15.8% on the X-plane with an aver-
with an average of 44.1%, and 2.4 to 5.4% on the Z-plane with an age of 12.8%, 8.8 to 15.6% on the Y-plane with an average of 12.1%,
average of 3.8%. Finally, for WWER-440 bioshielding concrete the and 11.8 to 12.1% on the Z-plane with an average of 12%.
D. Han et al. / Construction and Building Materials 163 (2018) 122–138 137

Table 17
The maximum surface dose rate of KHNP and concrete containers.

Concrete type AM RPV WWER-440 RPV WWER-440 concrete


X Y Z X Y Z X Y Z
KHNP Container 6.48 5.34 3.30 0.11 0.08 0.07 0.019 0.016 0.017
40NCA 1.897 1.408 0.220 0.042 0.036 0.0038 0.0027 0.0017 0.00018
40RCA 1.911 1.480 0.190 0.042 0.034 0.0033 0.0030 0.0016 0.00020
70NCA 1.817 1.619 0.107 0.044 0.036 0.0018 0.0021 0.0024 0.00020
70RCA 1.819 1.674 0.136 0.040 0.035 0.0017 0.0019 0.0023 0.00020

AM RPV WWER-440 RPV WWER-440 concrete results. Therefore, it is plausible to state that the numerical simu-
60% lation code has high reliability to evaluate radiation shielding per-
50% formance of concrete in comparison to an experimental method
40% and could be employed to predict radiation shielding properties
Ratio

of concrete. Meanwhile, the linear attenuation coefficients of RCA


30%
for 40 MPa are not significantly different when compared to NCA.
20% However, for the concrete samples with 70 MPa of compressive
10% strength, the RCA samples show slightly lower linear attenuation
0% coefficients than NCA. This might be due to lower density of RCA
40NCA 40RCA 70NCA 70RCA Average when compared to NCA.
Concrete type Finally, it has been found that the maximum surface dose rates
a) X-plane of the all concrete containers for both intermediate and low level of
radioactive waste in terms of gamma rays were turned out below
AM RPV WWER-440 RPV WWER-440 concrete the surface dose rate limit, 2 mSv/h, showing significantly less sur-
60%
face dose rates than the existing KHNP container. Based on these
50%
studies it can be concluded that concrete containing any virgin or
40% recycled coarse aggregate shows favorable properties as a shield-
Ratio

30% ing material; therefore it can be a useful material as transportable


20% packaging for radioactive waste.
10%
0% Acknowledgments
40NCA 40RCA 70NCA 70RCA Average
Concrete type This research project was funded by POSCO E&C R&D center in
b) Y-plane Korea. The authors acknowledge Ryan Schow and Steve Burnham
in UNEP for their contributions to establishing the test setups of
AM RPV WWER-440 RPV WWER-440 concrete radiation shielding.
10%

8% References

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