Abstract. In very intense electromagnetic fields, the vacuum refractive index is expected to be modified due
to nonlinear quantum electrodynamics (QED) properties. Several experimental tests using high intensity
lasers have been proposed to observe electromagnetic nonlinearities in vacuum, such as the diffraction or the
reflection of intense laser pulses. We propose a new approach which consists in observing the refraction,
i.e. the rotation of the waveplanes of a probe laser pulse crossing a transverse vacuum index gradient.
The latter is produced by the interaction of two very intense and ultra short laser pulses, used as pump
pulses. At the maximum of the index gradient, the refraction angle of the probe pulse is estimated to be
w0
0.2 × ( 10µm )−3 × 1J
I
picoradians, where I is the total energy of the two pump pulses and w0 is the minimum
waist (fwhm) at the interaction area. Assuming the most intense laser pulses attainable by the LASERIX
facility (I = 25 J, 30 fs fwhm duration, 800 nm central wavelength) and assuming a minimum waist of
w = 10µm (fwhm) (corresponding to an intensity of the order of 1021 W/cm2 ), the expected maximum
refraction angle is about 5 picoradians. An experimental setup, using a Sagnac interferometer, is proposed
to perform this measurement.
1 χm
2 Nonlinear properties of the electromagnetic M = χm H = B (5)
µ0 1 + χm
quantum vacuum
The optical refractive index is then given by
√
In classical electrodynamics, the electromagnetic proper- µ p
ties of the vacuum are described by two fundamental con- n= √ = (1 + χe )(1 + χm )
0 µ0
stants: the vacuum permittivity 0 and the vacuum per-
meability µ0 . In the presence of an eletric field E, the It is well established that in a high field regime, mate-
induced vacuum polarization D is given by rial media become optically nonlinear: the susceptibilities
are not constant but depend on the magnetic and electric
D = 0 E (1) fields applied to this medium.
X. Sarazin et al.: Refraction of light by light in vacuum 3
Since the early work by Heisenberg and Euler [1], it is In the following, we first calculate the gradient of the
predicted that the electromagnetic vacuum must also be- vacuum index induced by the interaction of the two pump
have as a nonlinear optical medium in presence of very in- pulses. We then calculate numerically the rotation angles
tense electromagnetic fields. The virtual electron-positron (the refraction angles) of the wave planes of the probe
fluctuations which are produced in the QED vacuum, are pulse, after having crossed the interaction area.
expected to induce nonlinear couplings between real elec-
tromagnetic fields. This modifies the interactions and prop-
agations of the fields and leads to modified Maxwell equa- 3.1 Variation of the vacuum refractive index induced
tions with a vacuum polarisation (similar to the ones in a by two counter propagating laser pulses
medium) given, at the lowest orders in the fields, by (see
e.g., Refs [2] and [11]) In the interaction area, the electromagnetic fields of each
pump pulse (labeled 1 and 2) are chosen to be two gaussian
P = ξ20 2(E 2 − c2 B 2 )E + 7(E · B)c2 B
wave packets of same amplitude:
M = −ξ20 c2 2(E 2 − c2 B 2 )B − 7(E · B)E
(6) E1 = A(x, y)F (z, t) cos[ω(t − z/c) − φ1 ] ux
with A(x, y)
B1 = F (z, t) cos[ω(t − z/c) − φ1 ] uy (8)
c
4α2 h̄3 m3
ξ= 4 5
' 3.35 10−30 (7)
45me c J E2 = A(x, y)F (z, −t) cos[ω(t + z/c) − φ2 ] uy
Because of this polarisation, the optical refractive in- A(x, y)
B2 = F (z, −t) cos[ω(t + z/c) − φ2 ] ux (9)
dex of the vacuum, for a light propagating in the presence c
of an external electromagnetic field, is no longer equal to with
1 but depends on the external field amplitude. 2
+y 2 )/∆2⊥ )
There are also QED corrections that include the spa- A(x, y) = A0 e−(2 ln2×(x (10)
tial and temporal derivatives of the fields E and B [12]. F (z, t) = e −(2 ln2×(t−z/c)2 /∆t2 )
(11)
However, as discussed in [11], the derivative corrections
are important when the wavelength of the light λ is com- where z is the axis of propagation, x and y are the trans-
parable to the Compton wavelength λC of the electron, verse axes, ux and uy are the unit vectors along x and
while the Heisenberg-Euler correction given in Equation 6 y respectively, ∆⊥ is the width (fwhm) of the transverse
is important when the electric field becomes comparable intensity profile, ∆t is the time width (fwhm) of the lon-
to the critical electric field Ec = m2 c3 /(eπh̄). More gener- gitudinal intensity profile, and t = 0 is arbitrarily defined
aly, it is shown in [11] that the derivative corrections are when the two pulses entirely overlap. For simplicity, we
negligible as long as (λC /λ)2 (4/π 3 )(E/Ec )2 . Since we will assume the phases φ1 and φ2 equal to 0 in the fol-
are studying a regime where the derivative corrections are lowing. Experimentaly, the two pump pulses have to be
negligible, we adopt the locally constant field approxima- sligthly tilted to prevent dangerous reinjection in the laser
tion and we consider only the Heisenberg-Euler correction amplifiers. However, we assume here that the tilt angle
given by Equation 6. between the two beam axes is small enough to be negligi-
ble as a first approximation. The transverse size, ∆⊥ , of
the pulses is also assumed to be constant at the interac-
3 Refraction of a probe pulse by the tion point and equal to the minimum waist. Indeed, the
interaction of two pump pulses diffraction effects can be neglected, as a first approxima-
tion, for laser pulses of duration lower than few hundreds
We study the configuration of two laser pulses (E1 ,B1 ) of femtoseconds and with a minimum waist larger than
and (E2 ,B2 ) with the same intensity and orthogonal lin- about 5 µm.
ear polarizations. These two pulses, named pump pulses, The amplitude A0 of the electromagnetic wave packets
propagate towards opposite directions along the same axis. depends on the total intensity I of the two pump pulses,
They cross each other at focus. The coupling of the two which is given by
fields induces an increase of the vacuum refractive in- Z
0 E12 B12
Z
dex which is proportional to the intensity of the fields. I=2 ( + )dxdydz = 20 E12 dxdydz (12)
Since the transverse intensity profile of the pump pulses 2 2µ0
is not uniform, a gradient of the vacuum index occurs At t = 0, we get
in the transverse direction of the propagation. A third ZZ +∞
pulse of lower energy (in the millijoule range), used as a I = 20 A20 e−(4 ln 2(x
2
+y 2 )/∆2⊥ )
dxdy
probe pulse, propagates simultaneously to one of the pump −∞
pulses, as illustrated in Figure 1, and crosses the trans- Z +∞
2 2
verse index gradient imprinted on the vacuum. The phase × e−(4 ln 2z /(c∆t) ) (cos(2ωz/c) + 1) dz
velocities in the probe pulse are gradually slower close to −∞
√
the interaction area, and the wave planes are gradually 2
2 π∆⊥ πc∆t 2 2
rotated. = 20 A0 √ 1 + e−ω ∆t /(4 ln 2) (13)
4 ln 2 2 ln 2
4 X. Sarazin et al.: Refraction of light by light in vacuum
With femtosecond laser pulses at 800 nm central wave- 3.2 Calculation of the refraction angles of a probe
2 2
length, e−ω ∆t /(4 ln 2) 1 and beam
√
2 4 ln 2 ln 2 I We assume that the probe pulse propagates at the same
A0 = √ (14) time, parallel to one of the pump pulses. The intensity of
0 π πc ∆2⊥ ∆t
the probe pulse (in the millijoule range) is about four or-
Assuming a waist of the laser beam at the interaction ders of magnitude smaller than that of the pump pulses.
area on the order of 10 µm (fwhm), and assuming a pulse Therefore its contribution to the index variation is ne-
duration of ∆t = 30 fs, the amplitude p A0 of the elec- glected. The refraction of the probe pulse is a pure wave
tric field of each pulse is A0 = 7.2 1012 I/(1 J) V/m. refraction effect. We can model it as the propagation of
This corresponds to an amplitude of the magnetic field of light rays (ray tracing) through the gradient of refractive
index in the transverse direction of propagation.
p
2.4 104 I/(1 J) Tesla.
The sum of the two pulses is given by All calculations are done assuming the performance of
the LASERIX facility, as given previously.
E = A(x, y)[F (z, t) cos(ω(t − z/c)) ux The calculation is performed numerically as follows.
+F (z, −t) cos(ω(t + z/c)) uy ] We first sample the pump pulse (E1 , B1 ) in x, y and z. We
then calculate at each point xi , yi , zi of the pulse, the total
A(x, y)
B= [F (z, −t) cos(ω(t + z/c)) ux index gradient ∂∆n(xi , yi , zi )/∂r in the transverse direc-
c tion r = xi ux + yi ux , integrated along the full crossing of
+F (z, t) cos(ω(t − z/c)) uy ] (15) the pulse with the second pump pulse (E2 , B2 ). Techni-
cally, since the terms of δnQED in the transverse directions
The fields are symmetric by inversion of x and y. Con- (x, y) and in the propagation direction (z, t) are indepen-
sequently we have E2 = c2 B2 and the nonlinear vacuum dant, we first calculate the integrated index ∆n(xi , yi , zi )
polarizations given by Eq. 6 become by integrating δnQED from t = −∆t to t = +∆t. Then we
P = 7ξ20 c2 (E · B) B calculate its gradient in the transverse direction r, given
by
M = 7ξ20 c2 (E · B) E (16)
Z +∆t !
By analogy with the susceptibilities of a medium given in ∂∆n(xi , yi , zi ) ∂
= δnQED (xi , yi , zi , t)dt (20)
Eq. 4 and 5, we can define the electric and magnetic sus- ∂r ∂r −∆t
ceptibilities χe0 and χm0 of the electromagnetic vacuum,
as For very small deflection, the integrated refraction angle
θr (xi , yi , zi ) in the transverse direction r is then given for
P · E = 0 χe0 E 2 each point (xi , yi , zi ) of the pulse by
1 χm0
M·B = B2 (17) ∂∆n(xi , yi , zi )
µ0 (1 + χm0 ) θr (xi , yi , zi ) = 2c∆t (21)
∂r
Combining Eq. 16 and 17, and at the first order (χe0 1
and χm0 1), one gets The integrated index ∆n(x, y, z = 0) and refraction
angle θr (x, y, z = 0), both calculated in the transverse
(E · B)2 plane z = 0, are presented as a function of x and y in Fig-
χe0 = 7ξ0 c2 ures 2 and 3, respectively. At the maximum of intensity
E2
(E · B)2 (x = y = 0), the integrated index is about 2 10−12 and at
χm0 = 7ξ0 = χe0 (18) the maximum of the index gradient, the integrated refrac-
B2
tion angle θr,max is about 5 picorad. The integrated index
The emergence of these susceptibilities leads to a variation ∆n(x, y, z = 0) calculated in the longitudinal plane y = 0
of the vacuum refractive index 1 + δnQED inside the laser is also presented as a function of the transverse coordinate
pulses, given at the first order in χe0 and χm0 , by x and the longitudinal coordinate z in Figure 4.
The refraction angle varies inversely as the cube of the
(E(x, y, z, t) · B(x, y, z, t))2 minimum waist w0 at the interaction area of the two pump
δnQED (x, y, z, t) = 7ξ0 c2 (19)
E 2 (x, y, z, t) pulses, and varies linearly with the total energy I of the
pump pulses, as
We can verify a posteriori that the increase of the vac-
uum refractive index is maximal when the two counter- w0 −3 I
propagating pump fields (E1 ,B1 ) and (E2 ,B2 ) have the θr,max = 2 10−13 × ( ) × radians (22)
10µm 1J
same intensity. This is why we propose to use that con-
figuration. As mentioned in the introduction, since the In theory, the refraction angle is insensitive to the duration
measurement of the waveplanes rotation within the in- of the pump pulses since the refraction is integrated along
tense pump pulses is experimentaly unrealistic, we use a all the longitudinal profile of the pulses. However, a waist
third probe pulse with a much lower intensity to probe of the order of 10 µm must be maintained in the inter-
the vacuum index gradient. action area. Therefore the longitudinal size of the pulses
X. Sarazin et al.: Refraction of light by light in vacuum 5
2.5
y (µm)
y (µm)
10 10 5
2.25
7.5 2 7.5
4
5 1.75 5
3
0 1.25 0
-2.5 1 -2.5
2
-5 0.75 -5
0.25
-10 -10
0 0
-10 -7.5 -5 -2.5 0 2.5 5 7.5 10 -10 -7.5 -5 -2.5 0 2.5 5 7.5 10
x (µm) x (µm)
Fig. 2. The integrated index ∆n(x, y, z = 0) (×1012 ) calcu- Fig. 3. The refraction angle θr (x, y, z = 0) (×1012 radians)
lated in the transverse plane z = 0, as a function of the trans- calculated in the transverse plane z = 0, as a function of the
verse coordinates x and y. The total energy of the two pump transverse coordinates x and y. At the maximum of the index
pulses is 25 J, the duration of each pulse is 30 fs (fwhm) and gradient (r ' 5µm), the refraction angle is about 5 10−12 rad.
the minimum waist is 10 µm at the focus, corresponding to an Computation is done with same conditions as for Fig. 2.
intensity of the order of 1021 W/cm2 .
∆n(y=0) × 1012
must be smaller than few tens of micrometers in order to 2.5
x (µm)
femtoseconds.
7.5 2
5 1.75
statistical error on the number of detected photons NB in as small as 0.1 picoradians have been detected with con-
the region of interest (∆r/2 < |r| < ∆r/2 + a). Noting tinuous laser beams with standard techniques using quad-
N0 the number of photons of the initial probe pulse before rant photodetectors, some limitations appear with ultra
entering the Sagnac interferometer, and Nshot the number short and intense pulses. In order to overpass these lim-
of repetitions of laser shots, then NB = a/∆r×2 N0 Nshot , itations, we propose to use a Sagnac interferometer, for
and the relative uncertainty of the background is which the measurement of the refraction is performed in
p p p its dark port, thus allowing high intensity probe pulses.
∆IB /IB = 1/ NB = ( ∆r/a)/( N0 Nshot ) (26) We estimate that the attenuation factor of the interfer-
ometer must be of the order of 10−6 in order to detect
The sensitivity of the measurement, given by the ratio of a signal larger than the background fluctuation after 104
the signal over background fluctuation, is LASERIX shots (correponding to about 1 day of measure-
ment).
IS δ p
=√ N0 Nshot (27)
∆IB a∆r
Acknowledgments
Assuming a beam diameter ∆r = 1 mm, a width of the
profile edge a = ∆r/10 = 100 µm, a repetition of laser The authors thank J. Haı̈ssinski for fruitful discussions on
shots Nshot = 104 (corresponding to about one day of this paper. The authors also thank L-Acoustics Company
measurement with the LASERIX repetition rate of 0.1 Hz), for their financial support for building a Sagnac interfer-
and a transverse displacement δ = 10−11 m (correspond- ometer prototype. We are also grateful to one of the refer-
ing to a refraction angle θr = 10 prad and a focal length ees who allowed us to clarify and complete our proposal.
f = 1 m), the ratio is
IS p
= 3.10−6 N0 (28) References
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ciples of a new and complementary method which consists
in observing the refraction, i.e. the rotation of the wave-
planes of a probe laser pulse crossing a transverse vacuum
index gradient. The latter is produced by the interaction
of two counter-propagating very intense and ultra short
laser pulses, used as pump pulses. The transverse gradient
of the vacuum refractive index is calculated and the refrac-
tion angle of the probe pulse crossing this index gradient
w0 −3 I
is shown to be 0.2×( 10µm ) × 1J picoradians at the max-
imum. This corresponds, for the most intense laser pulses
attainable today by the LASERIX facility (I = 25 J) and
with a minimum waist of w0 = 10 µm at the focus, to 5 pi-
coradians at the maximum. Although angular deviations